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    Bismuth(III) oxide and boron(III) oxide substitution in bismuth-boro-zinc glasses: a focusing in nuclear radiation shielding properties
    (ELSEVIER GMBH, 2023) Almisned, Ghada; Bilal, Ghaida; Şen Baykal, Duygu; Ali, Fatema T.; Kılıç, G.; Tekin, Hüseyin Ozan
    Doping the glass structure with Bi2O3 `is known to increase structural stability, and to drastically alter physical parameters including density and molar volume. The goal of this work was to assess the nuclear radiation attenuation competences of several types of glasses based on the xBi2O3-(70x)B2O3-8BaO-16ZnO-5.5SiO2- 0.5Sb2O3 system. In order to determine the requisite gamma shielding parameters, as well as effective conductivity at 300 K and buildup factors, five different glasses with varied Bi2O3 concentration (i.e., from 10 mol.% to 30 mol.%) were examined thoroughly. These critical parameters were determined using the Phy-X/PSD program. In addition, factors such as half value layer (HVL), tenth value layer (TVL), and mean free path (mfp) were examined over a wide energy range of 0.015-15 MeV. The findings revealed that the amount of Bi2O3 reinforced in each sample is critical in determining the samples' shielding abilities. The linear attenuation coefficients (mu) and mass attenuation coefficient (mu m) values were reported in the highest level for the sample with the highest Bi2O3 content. For glass sample A5, the lowest mean free path, half value layer, and tenth value layer values were also reported. The effective conductivity and effective atomic number had an inverse relationship with photon energy, meaning that as energy increased, the effective conductivity and effective atomic number declined fast, especially in low-energy regions. The greatest values for both parameters were found in glass sample A5. Furthermore, the exposure buildup factor and energy absorption buildup factor values for glass sample A5 were the lowest. A5 glass sample with the chemical composition 30Bi2O3-(70 30) B2O3-8BaO-16ZnO-5.5SiO2- 0.5Sb2O3 and a density of 5.8391 g/ cm3 was found to have exceptional gamma-ray attenuation qualities, according to our findings. It can be concluded that the prospective attributes of Bi2O3-doped glass systems and associated glass compositions would be beneficial for scientific community in terms of providing a clearer view for some advanced applications of these glass types.
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    Gadolinium-tungsten-boron trioxide glasses: A multi-phase research on cross-sections, attenuation coefficients, build-up factors and individual transmission factors using MCNPX
    (Elsevier, 2022) ALMisned, Ghada; Sen Baykal, Duygu; Ali, Fatema T.; Bilal, Ghaida; Kılıç, Gökhan; Tekin, Hüseyin Ozan
    The oxide of the rare earth element gadolinium has the chemical formula Gd2O3. Also known as gadolinium sesquioxide, gadolinium trioxide, and Gadolinia, gadolinium oxide. In this study, various types of fundamental cross-sections, attenuation coefficients, build-up factors and individual transmission factors of high density gadolinium-tungsten-boron trioxide glasses with a chemical composition of (70-x)WO3-xGd2O3 –30B2O3 (where x: 17.5, 20.0, 22.5, 25.0 and 27.5 mol%) are determined using advanced Monte Carlo methods. In addition, gamma transmission factors (TFs) for a range of medical and industrial radioisotopes were calculated using MCNPX (version 2.7.0) Monte Carlo code. The investigated glasses were classified Gd17.5, Gd20.0, Gd22.5, Gd25.0, and Gd27.5 in accordance with xGd2O3. Our findings suggest that the Gd27.5 sample (with highest of Gd2O3 content mol. %) has possessed the maximum linear (µ) and mass (µ/?) attenuation coefficients at all gamma-ray energies investigated. The coded glass sample Gd27.5 is achieved the maximum effective atomic number (Zeff) and effective electron density (Neff) owing its superior attenuation properties. In terms of build-up factors, increasing the concentration of xGd2O3 in glasses is decreased the EBF and EABF values for all mean free path values (0.5–40 mfp). At a thickness of 3 cm, the lowest transmission factor (i.e., highest attenuation) was verified for all Gd17.5-Gd27.5 glasses investigated. Consequently, the Gd27.5 sample exhibits superior radiation shielding properties for a large range of photon energy and various medical and industrial radioisotope energies. © 2022 Elsevier GmbH
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    Gamma, neutron, and heavy charged ion shielding properties of Er3+-doped and Sm3+-doped zinc borate glasses
    (De Gruyter Open Ltd, 2022) Tekin, Hüseyin Ozan; Almisned, Ghada; Zakaly, Hesham M.H.; Zamil, Abdallah; Khoucheich, Dalia; Bilal, Ghaida; Al-Sammarraie, Lubna; Issa, Shams A.M.; Al-Buriahi, Mohammed Sultan; Ene, Antoaneta
    This study aimed to investigate the nuclear radiation shielding properties of erbium (Er)-reinforced and samarium (Sm)-reinforced borate glasses. In the 0.015-15 MeV photon energy range, attenuation coefficients, as well as half-value layer tenth-value layers, and the mean-free path have been calculated. Additionally, effective, and equivalent atomic numbers, effective atomic weight, electron density, and exposure and energy absorption build-up factors were also calculated. To evaluate the overall nuclear radiation attenuation competencies of Er-rich and Sm-rich glasses, effective removal cross-section values for fast neutrons and projected range/mass stopping power values for alpha and proton particles were also determined. The glass sample BZBEr2.0 had the highest linear and mass attenuation coefficients (? and ?m), effective conductivity (Ceff), the effective number of electrons (Neff), and effective atomic number (Zeff) values as well as the lowest half-value layer (T1/2), tenth value layers (T1/10), mean free path (?), exposure build-up factor, and energy absorption build-up factor values. ?m values were reported as 2.337, 2.556, 2.770, 2.976, 2.108, 2.266, 2.421, 2.569, and 2.714 for BZBEr0.5, BZBEr1.0, BZBEr1.5, BZBEr2.0, BZBSm0.0, BZBSm0.5, BZBSm1.0, BZBSm1.5, and BZBSm2.0 glass samples at 0.06 MeV, respectively. The results showed that Er has a greater effect than Sm regarding the gamma-ray shielding properties of borate glasses. The results of this investigation could be used in further investigations and added to older investigations with the same aim, to aid the scientific community in determining the most appropriate rare-earth additive, to provide adequate shielding properties based on the requirement. © 2022 Huseyin Ozan Tekin et al., published by De Gruyter.